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Review Tier 2

A focused review on recycling and hydrolysis techniques of polyethylene terephthalate

This review examines techniques for recycling polyethylene terephthalate (PET), one of the most common plastics found as microplastic pollution. Chemical recycling through hydrolysis shows the most promise for breaking PET back into its original building blocks for reuse. Improving PET recycling is important because reducing plastic waste at the source is one of the most effective ways to decrease microplastic contamination in the environment.

2023 Polymer Engineering and Science 154 citations
Article Tier 2

Polymer Chemistry: A primer to enzymatic polymer degradation

This review primer covers how enzymes can be used to biodegrade polymers, with applications for chemical recycling of plastics and removal of microplastic debris from the environment. Enzymatic degradation offers a targeted, environmentally friendly approach to breaking down persistent plastic polymers at the source.

2023 Nachrichten aus der Chemie
Article Tier 2

Application of Different Chemical Recycling for Plastics

This review examines chemical recycling methods for plastic waste as alternatives to mechanical recycling, focusing on depolymerization via solvolysis, pyrolysis, and purification processes applicable to PET, polyurethane, and polystyrene. The authors discuss how these approaches convert polymer waste back into feedstock monomers that can be repolymerized, addressing value degradation and sorting limitations inherent to mechanical recycling.

2022 Highlights in Science Engineering and Technology 1 citations
Article Tier 2

Research progress on chemical depolymerization and upcycling of PET waste plastics

This review examines recent advances in chemical methods for breaking down polyethylene terephthalate (PET) waste plastics into useful raw materials. Researchers surveyed techniques including glycolysis, methanolysis, hydrolysis, and aminolysis that can convert PET back into monomers for reuse. The study highlights chemical depolymerization as a promising approach to reduce plastic pollution while recovering valuable materials from waste.

2025 Chinese Science Bulletin (Chinese Version) 1 citations
Article Tier 2

Current Advances and Challenges in Chemical Recycling of Polymeric Materials

This review examines current advances and remaining challenges in chemical recycling of polymeric materials as an alternative to mechanical recycling, which degrades material properties with repeated cycling. The authors discuss the high efficiency and simpler preprocessing requirements of chemical recycling methods against a backdrop of approximately 150 million metric tonnes of annual global plastic waste generation.

2023 Preprints.org 4 citations
Article Tier 2

Structural decay of poly(ethylene terephthalate) by enzymatic degradation

Researchers examined the structural decay of poly(ethylene terephthalate) through enzymatic degradation as a sustainable recycling strategy, finding this approach requires neither energy nor harsh solvents, offering a promising path for addressing microplastic pollution from PET products.

2025 Polymer Journal
Article Tier 2

Enzymatic Degradation of PET plastic

This study tested commercial-grade enzymes for degrading PET plastic and found that enzymatic degradation was effective at laboratory scale but faced challenges for real-world application. Scaling up enzymatic PET recycling could reduce the persistence of plastic waste that eventually fragments into microplastics in the environment.

2023 ARPHA Conference Abstracts
Article Tier 2

An Overview of the Non-Energetic Valorization Possibilities of Plastic Waste via Thermochemical Processes

This review surveys non-energetic valorization options for plastic waste through chemical recycling, covering solvolysis, enzymatic depolymerization, and catalytic cracking pathways that recover monomers or chemical feedstocks. The authors compare process maturity and economic viability, identifying PET and nylon depolymerization as the most commercially advanced chemical recycling routes.

2024 Materials 4 citations
Article Tier 2

Development of Enzyme-Based Approaches for Recycling PET on an Industrial Scale

This paper reviews the development of enzyme-based methods for breaking down PET plastic (used in bottles and packaging) at an industrial scale. While enzymatic recycling is a promising solution to plastic waste, current methods are still too slow and costly for widespread use. Improving these technologies could help reduce the enormous amount of PET entering the environment and breaking down into microplastics.

2024 Biochemistry 22 citations
Article Tier 2

Light-driven polymer recycling to monomers and small molecules

Researchers reviewed how sunlight can be harnessed to chemically break down plastic waste into reusable molecules, offering a lower-energy alternative to heat-based recycling methods like pyrolysis. While still limited to certain plastic types, light-driven recycling shows promise for converting hard-to-recycle plastics into valuable chemical building blocks.

2024 Nature Communications 76 citations
Article Tier 2

On technological solutions for recycling of recycling of polymer waste: A review

This paper is not directly about microplastics; it reviews technological approaches to recycling polymer waste — mechanical, chemical, and energy-based methods — and analyzes their economic and environmental trade-offs. Better plastic recycling technology is relevant to microplastic prevention insofar as it reduces the amount of plastic that degrades into environmental microplastic particles.

2024 E3S Web of Conferences 2 citations
Article Tier 2

Process parameter optimization for waste polyethylene terephthalate bottle depolymerization using neutral hydrolysis

Researchers optimized process parameters for the neutral hydrolysis depolymerization of waste polyethylene terephthalate (PET) bottles as a chemical recycling strategy to address growing plastic waste accumulation in landfills. The study identified key conditions that improve depolymerization efficiency, offering a pathway to recover high-quality monomers from post-consumer PET.

2024 Research Square (Research Square) 1 citations
Article Tier 2

Microbial Degradation of Plastic Polymers

This review examines microbial degradation pathways for common synthetic plastics including polyethylene, polypropylene, polystyrene, PVC, polyurethane, and PET, describing how mechanical and biological processes fragment plastics into microplastics and how microorganisms can be leveraged to address plastic pollution in aquatic and terrestrial environments.

2025
Article Tier 2

Biodegradation of Microplastic: A Sustainable Approach

This review examines biological approaches to microplastic degradation, covering microorganisms and enzymes capable of breaking down common plastic polymers such as PET and polyethylene. Biodegradation could offer a sustainable path to reducing microplastic accumulation in soil, water, and marine environments.

2023 International Journal of Current Microbiology and Applied Sciences
Article Tier 2

Enzymatic Remediation of Polyethylene Terephthalate (PET)–Based Polymers for Effective Management of Plastic Wastes: An Overview

Enzymatic approaches for remediating PET-based plastic waste were reviewed, covering PETase and related enzymes that can break PET into reusable monomers. Enzyme engineering strategies to improve thermostability and catalytic efficiency are discussed as a pathway to scalable biological PET recycling.

2020 Frontiers in Bioengineering and Biotechnology 193 citations
Article Tier 2

Comparative Reactivity of Different Polyols in the PET Saponification Process

Researchers investigated the chemical depolymerization of PET plastic using different polyols and glycerol, finding that reaction conditions like temperature and chemical ratios controlled the molecular weight of the resulting oligomers. Ethylene glycol enabled rapid, complete PET breakdown within 30 minutes. Chemical recycling of PET through saponification could reduce the amount of PET that fragments into microplastics in the environment.

2023 AppliedChem 1 citations
Article Tier 2

Biodegradation of Plastic and the Role of Microbial Enzymes in Plastic Waste Management

This review examines how microbial enzymes, particularly PET hydrolases and oxidative enzymes, can depolymerize and break down common plastic polymers through biological degradation. The study suggests that enzymatic approaches to plastic waste management offer a promising complement to mechanical and chemical recycling, though optimizing enzyme activity and scaling up the process remain key challenges.

2026 International Journal of Education Management and Technology
Article Tier 2

Recent Advances in the Chemobiological Upcycling of Polyethylene Terephthalate (PET) into Value-Added Chemicals

This review covers recent advances in biological and chemical upcycling of PET plastic waste into value-added chemicals, examining degradation pathways including pyrolysis, gasification, and enzymatic depolymerization that break PET into monomers for use as bioconversion substrates.

2022 Journal of Microbiology and Biotechnology 39 citations
Article Tier 2

Enzymatic PET Degradation

This review examines enzymatic degradation of PET (polyethylene terephthalate), the plastic used in bottles and polyester clothing, as a promising pathway for breaking down this persistent polymer. Advances in engineering more efficient PET-degrading enzymes could enable industrial-scale biological recycling and reduce the environmental accumulation of PET microplastics.

2019 CHIMIA International Journal for Chemistry 50 citations
Article Tier 2

Polyesters and deep eutectic solvents: From synthesis through modification to depolymerization

This review examines how deep eutectic solvents, a class of greener chemical alternatives, can be used throughout the lifecycle of polyester plastics, from manufacturing to recycling. Researchers found these solvents show promise for catalyzing plastic depolymerization in closed-loop recycling systems at lower cost than traditional methods. The study is relevant to microplastic pollution because improving plastic recycling could help reduce the amount of polyester waste that breaks down into microplastics in the environment.

2025 Progress in Polymer Science 15 citations
Article Tier 2

Microbial enzymes for the recycling of recalcitrant petroleum‐based plastics: how far are we?

This review examines the progress in identifying microbial enzymes capable of breaking down petroleum-based plastics like polyethylene, polystyrene, polyurethane, and PET. Researchers highlight recent advances in using polyester-degrading enzymes to recover raw materials from PET waste through biocatalytic recycling. The study discusses the potential and remaining challenges of using biological approaches to address the growing global problem of plastic waste accumulation.

2017 Microbial Biotechnology 788 citations
Article Tier 2

Light-Driven Polymer Recycling to Monomers and Small Molecules

Researchers developed and reviewed light-driven photochemical methods for recycling polymers back into monomers and small molecules, presenting an energy-efficient alternative to high-temperature pyrolysis and other chemical recycling approaches. The study shows that photocatalytic depolymerization can achieve selective bond cleavage at lower energy inputs, advancing the viability of circular polymer chemistry.

2024 1 citations
Article Tier 2

Degradation and Recycling of Polymer Materials

This review synthesizes research on the degradation and recycling of polymer materials, covering microplastic formation, recycling strategies, and plastic degradation mechanisms as responses to the significant environmental damage caused by discarded plastics in ocean and other ecosystems.

2025
Article Tier 2

Optimization of Pressurized Alkaline Hydrolysis for Chemical Recycling of Post-Consumer PET Waste

This study optimized pressurized alkaline hydrolysis conditions for chemically recycling post-consumer PET waste into its constituent monomers, demonstrating a pathway to improve the efficiency of PET depolymerization.

2024 Materials 8 citations