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Accelerated aging behavior of degradable and non-degradable microplastics via advanced oxidation and their adsorption characteristics towards tetracycline
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Researchers compared how biodegradable polylactic acid and conventional polystyrene microplastics age when exposed to advanced oxidation processes, and how aging changes their ability to adsorb the antibiotic tetracycline. They found that polylactic acid degraded more quickly and developed more surface changes during aging, leading to increased antibiotic adsorption. The findings suggest that as biodegradable plastics break down in the environment, they may become more effective at concentrating and transporting chemical contaminants.
The increasing global utilization of biodegradable plastics due to stringent regulations on traditional plastics has caused a significant rise in microplastic (MPs) pollution in aquatic ecosystems from biodegradable products. However, the environmental behavior of biodegradable MPs remains inadequately elucidated. This study explored the aging processes of polylactic acid (PLA) and polystyrene (PS) under a heat-activated potassium persulfate (KSO) system, as well as their adsorption characteristics towards tetracycline (TCs). In comparison to PS, the surface structure of PLA experienced more pronounced changes over aging, exhibiting evident pits, cracks, and fragmentation. The carbonyl index (CI) and oxygen/carbon ratio (O/C) of PS displayed exponential growth over time, whereas the values for PLA showed linear and exponential increases, respectively. The adsorption capacity of TCs by PS and PLA aged for 6 days increased from 0.312 mg‧g and 0.457 mg‧gfor original PS and PLA, respectively, to 0.372 mg‧g and 0.649 mg‧g. Meanwhile, the adsorption rate (k values) for TCs decreased by 42.03 % for PS and 79.64 % for PLA compared to their initial values. The findings indicated that biodegradable PLA-MPs may exhibit higher tetracycline carrying capacities than PS, potentially increasing environmental and organismal risks, particularly in view of aging effects.
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Aging characteristics of degradable and non-biodegradable microplastics and their adsorption mechanism for sulfonamides
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Researchers investigated how aging processes affect the ability of degradable and non-biodegradable microplastics to adsorb sulfonamide antibiotics in aquatic environments. The study found that aging increased the hydrophilicity and polarity of microplastics, boosting the adsorption capacity of polylactic acid by up to 3.18 times, suggesting that weathered microplastics may pose greater ecological risks as carriers of co-existing contaminants.
Adsorption/desorption behavior of degradable polylactic acid microplastics on bisphenol A under different aging conditions
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Researchers studied how different types of UV-simulated aging affect the ability of polylactic acid microplastics to adsorb and release bisphenol A. The study found that aging conditions changed the surface properties of the biodegradable plastic, altering its interaction with this common environmental contaminant. The findings suggest that even biodegradable microplastics can act as carriers of harmful chemicals depending on their degradation state.
UV and chemical aging alter the adsorption behavior of microplastics for tetracycline
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Researchers found that UV and chemical aging significantly increased microplastics' capacity to adsorb tetracycline, with biodegradable PBAT showing more dramatic changes in surface properties and adsorption behavior compared to conventional plastics like polystyrene and polyethylene.
Behavior and mechanisms of ciprofloxacin adsorption on aged polylactic acid and polyethlene microplastics
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Researchers investigated how aging affects the adsorption of the antibiotic ciprofloxacin on polylactic acid and polyethylene microplastics, finding that aged plastics showed significantly enhanced adsorption capacity due to physicochemical surface changes.
Impact of sequential UV-aging of microplastics on the fate of antibiotic (tetracycline) in riverine, estuarine, and marine systems
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Researchers studied how sequential UV aging of polystyrene, polypropylene, and polyethylene microplastics, which mimics natural weathering, affects their ability to adsorb the antibiotic tetracycline under different water chemistry conditions. They found that aged microplastics adsorbed significantly more tetracycline than pristine particles, with the effect varying by water type and plastic polymer. The study suggests that as microplastics weather in the environment, they may become increasingly effective at carrying antibiotic contaminants.
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