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Adsorption of lead(II) onto PE microplastics as a function of particle size: Influencing factors and adsorption mechanism

Chemosphere 2022 90 citations ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count. Score: 60 ? 0–100 AI score estimating relevance to the microplastics field. Papers below 30 are filtered from public browse.
Thi-Bao-Chau Ho, Shu‐Ling Hsieh, Wei‐Hsin Chen, Shu‐Ling Hsieh, Shu‐Ling Hsieh, Thanh-Binh Nguyen, Wei‐Hsin Chen, Thanh-Binh Nguyen, Thi-Bao-Chau Ho, Thi-Bao-Chau Ho, Thanh-Binh Nguyen, Wei‐Hsin Chen, Wei‐Hsin Chen, Chiu‐Wen Chen, Thi-Bao-Chau Ho, Thi-Bao-Chau Ho, Thi-Bao-Chau Ho, Chin‐Pao Huang, Thi-Bao-Chau Ho, Thi-Bao-Chau Ho, Chiu‐Wen Chen, Shuchen Hsieh, Shu‐Ling Hsieh, Shu‐Ling Hsieh, Shuchen Hsieh, Chiu‐Wen Chen, Chin‐Pao Huang, Shu‐Ling Hsieh, Chin‐Pao Huang, Wei‐Hsin Chen, Shu‐Ling Hsieh, Cheng–Di Dong, Chiu‐Wen Chen, Chiu‐Wen Chen, Chiu‐Wen Chen, Wei‐Hsin Chen, Thanh-Binh Nguyen, Thanh-Binh Nguyen, Chin‐Pao Huang, Cheng–Di Dong Wei‐Hsin Chen, Thanh-Binh Nguyen, Wei‐Hsin Chen, Shuchen Hsieh, Wei‐Hsin Chen, Wei‐Hsin Chen, Cheng–Di Dong Chiu‐Wen Chen, Wei‐Hsin Chen, Chiu‐Wen Chen, Chiu‐Wen Chen, Cheng–Di Dong Cheng–Di Dong Shuchen Hsieh, Cheng–Di Dong, Wei‐Hsin Chen, Chiu‐Wen Chen, Chin‐Pao Huang, Cheng–Di Dong, Cheng–Di Dong, Shu‐Ling Hsieh, Cheng–Di Dong, Wei‐Hsin Chen, Shuchen Hsieh, Shuchen Hsieh, Shu‐Ling Hsieh, Chiu‐Wen Chen, Chiu‐Wen Chen, Cheng–Di Dong, Cheng–Di Dong, Cheng–Di Dong, Cheng–Di Dong, Wei‐Hsin Chen, Wei‐Hsin Chen, Chin‐Pao Huang, Cheng–Di Dong Cheng–Di Dong Cheng–Di Dong Cheng–Di Dong Shuchen Hsieh, Shuchen Hsieh, Shuchen Hsieh, Shuchen Hsieh, Cheng–Di Dong, Shu‐Ling Hsieh, Cheng–Di Dong, Chiu‐Wen Chen, Cheng–Di Dong Shu‐Ling Hsieh, Chiu‐Wen Chen, Wei‐Hsin Chen, Cheng–Di Dong Chiu‐Wen Chen, Cheng–Di Dong Thanh-Binh Nguyen, Cheng–Di Dong, Cheng–Di Dong Cheng–Di Dong, Cheng–Di Dong Chiu‐Wen Chen, Cheng–Di Dong, Cheng–Di Dong, Cheng–Di Dong Chiu‐Wen Chen, Cheng–Di Dong, Cheng–Di Dong Cheng–Di Dong

Summary

Researchers studied how lead ions attach to polyethylene microplastics of different sizes in water. They found that smaller microplastic particles had greater capacity to adsorb lead, primarily through chemical bonding mechanisms like hydrogen bonding and surface complexation. The findings suggest that microplastics in the environment can act as carriers for toxic heavy metals, with smaller particles posing a greater risk.

Polymers

The adsorption of Pb ions, on high-density polyethylene (PE) microplastics (MPs) with the diameter of 48-500 μm, was examined in this study. According to the Langmuir isotherm, MP of the smallest size, 48 μm, had the greatest adsorption capacity of 0.38 μmol g. The mechanism of Pb ions adsorption onto PE MPs was chemical adsorption, in particular, hydrogen bonding and surface complexation. Pb adsorption onto PE particles was proceeded at a rapid rate, as predicted by the pseudo-second-order rate model (R > 0.99). The PE 48 μm had the maximum adsorption capacity of 0.44 μmol g-1 (or 0.2 mol m) at pH 5. While humic acid can operate as a bridging agent, boosting heavy metal adsorption on the surface of PE MPs, fulvic acid has the reverse effect. The findings indicated that PE particles may serve as a carrier of heavy metals in the aquatic environment, posing perceived risks to the environment and public health.

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