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Real-time detection of label-free submicron-sized plastics using flow-channeled differential interference contrast microscopy

2023 1 citation ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count. Score: 40 ? 0–100 AI score estimating relevance to the microplastics field. Papers below 30 are filtered from public browse.
Jae Hun Kim, Jae Hun Kim, Jiyun Han, Subeen Park, Subeen Park, Mingizem Gashaw Seid, Byoungho Park, Soo Hyun Lee, Hyung Min Kim, Jae Sang Lee, Seok Won Hong

Summary

Researchers developed differential interference contrast microscopy for real-time label-free detection of submicron plastics in water, overcoming bright-field microscopy limits.

Polymers

Abstract Owing to the surge in plastic waste generated during the COVID-19 pandemic, concern regarding microplastic pollution in aqueous environments is increasing. Since sub-micron plastics can accumulate in the human body, their real-time detection in water is necessary. However, the decrease in the scattering cross-section of small polystyrene (PS) particles in aqueous media precludes detection by bright-field microscopy. To address this problem, we propose and demonstrate a differential interference contrast (DIC) system that incorporates a magnification-enhancing system to detect PS beads in aqueous samples. To detect micron-scale and sub-micron-scale PS beads in the stationary and mobile phases, a microfluidic chip was designed considering the imaging depth of focus and flow resistance. PS beads of various sizes flowing in deionized and tap water at varying speeds were quantitatively observed under Static and Flow conditions. The real-time detection and quantification of PS beads of size ≥ 200 nm at a constant flow rate in water was successful. It was also possible to classify two different sizes, 2 µm and 750 nm, in a mixed solution. Thus, the proposed novel method can significantly reduce the analysis time and improve the size-detection limit. The proposed DIC microscopy system can be coupled with Raman or IR spectroscopy in future study for chemical composition analysis.

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