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Enhancement of photodegradation of polyethylene with adsorbed polycyclic aromatic hydrocarbons under artificial sunlight irradiation
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Researchers showed that polycyclic aromatic hydrocarbons (PAHs) adsorbed onto polyethylene plastic act as photocatalysts that accelerate the photodegradation of the plastic in marine environments, increasing microplastic production from plastic waste contaminated with hydrophobic organic pollutants.
The photodegradation of plastic waste produces microplastics (MPs) in marine environments. Plastics can adsorb hydrophobic organic pollutants such as polycyclic aromatic hydrocarbons (PAHs) and can be transported over long distances. However, the impact of adsorbed pollutants on the photodegradation remains unknown. Here, we show that adsorbed PAHs act as photocatalysts that promote the photodegradation of polyethylene. Upon light irradiation, coloration and surface degradation of the PAH-adsorbed polyethylene sheets were observed, indicating that the PAH-adsorbed polyethylene sheets are less resistant to light. Furthermore, fluorene, phenanthrene, anthracene, benzo[a]anthracene, benzo[a]pyrene, and indeno[1,2,3-cd]perylene adsorbed on polyethylene MP exhibited lower photodegradation rates than the aqueous phase. These results indicate that these PAHs can act as photocatalysts; their role of PAHs may have two adverse effects on marine environment. First, enhanced photodegradation of plastic waste increased the production of MPs. Second, the lifetime of PAHs is extended, thereby enhancing PAHs pollution in marine environments.
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Researchers investigated the photolysis of polycyclic aromatic hydrocarbons adsorbed onto polyethylene microplastics under natural sunlight conditions, finding that PAH concentrations on microplastic surfaces decreased over time due to photodegradation. The study provides first data on the environmental fate of PAH-microplastic complexes under realistic solar irradiation.
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Researchers studied the sorption of polycyclic aromatic hydrocarbons (PAHs) onto weathered polypropylene microplastics in seawater, finding that weathering increased surface area and adsorption capacity compared to pristine particles. This suggests environmental aging enhances microplastics as vectors for hydrophobic pollutants.
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