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Convenient Size Analysis of Nanoplastics on a Microelectrode

Analytical Chemistry 2024 7 citations ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count.
Xuan He, Xin Xie, Juan Xiang, Minghui Yang

Summary

Researchers developed a microelectrode-based method for size analysis of nanoplastics in suspension, enabling convenient, rapid characterization without specialized nanoparticle tracking instruments. The method accurately measured particle size distributions down to the nanometer range and showed potential for integration into routine environmental monitoring workflows.

Polymers

Chemical recycling is a promising approach to reduce plastic pollution. Timely and accurate size analysis of produced nanoplastics is necessary to monitor the process and assess the quality of chemical recycling. In this work, a sandwich-type microelectrode sensor was developed for the size assessment of nanoplastics. β-Mercaptoethylamine was modified on the microelectrode to enhance its surface positive charge density. Polystyrene (PS) nanoplastics were captured on the sensor through electrostatic interactions. Ferrocene was used as an electrochemical beacon and attached to PS via hydrophobic interactions. The results show a nonlinear dependence of the sensor's current response on the PS particle size. The size resolving ability of the microelectrode is mainly attributed to the small size of the electrode and the resulting attenuation of the electric field strength. For mixed samples with different particle sizes, this method can provide accurate average particle sizes. Through an effective pretreatment process, the method can be applied to PS nanoplastics with different surface properties, ensuring its application in evaluating different chemical recycling methods.

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