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Influence of biodegradable plastics on the generation of disinfection byproducts in the chlorination process
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This study investigated how biodegradable plastics influence the generation of dissolved organic matter and its downstream effects on water quality and treatment processes. The findings show that biodegradable polymers can release organic compounds that complicate wastewater treatment compared to conventional plastics.
Biodegradable plastics (BPs) have seen a continuous increase in annual production and application due to their environmentally sustainable characteristics. However, research on the formation of disinfection byproducts (DBPs) from biodegradable microplastics (BMPs) during chlorination is limited, and the effects of aqueous solution chemistry on this process have yet to be explored. Therefore, two biodegradable microplastics, polylactic acid (PLA) and polybutylene adipate terephthalate (PBAT), were investigated in this study to examine the changes in their physicochemical properties before and after chlorination, and the formation of DBPs under different environmental conditions. The results showed that PLA was more chlorine-responsive, and generated more DBPs. The pH converted some of the intermediates into more stable DBPs by affecting the concentration of HClO and base-catalyzed reactions, whereas ionic strength slightly reduced DBP concentration by ion adsorption and promoting the aggregation of BMPs. Finally, since PLA has a slightly greater volume of mesopores and micropores compared to PBAT, it may more effectively adsorb DBP precursors beyond natural organic matter (NOM), such as some anthropogenic pollutants, thus potentially decreasing the formation of chlorinated DBPs in surface water. This research explored the potentiality for DBP formation by BMPs under different water quality conditions during the disinfection process, which is useful for assessing the environmental hazards of BMPs.
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Researchers investigated how microplastics affect disinfection byproduct formation during chlorination of natural organic matter in water treatment, finding that the presence of microplastics can influence the generation of potentially harmful DBPs.
Insight into the dynamic transformation properties of microplastic-derived dissolved organic matter and its contribution to the formation of chlorination disinfection by-products
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Researchers studied how dissolved organic matter released from microplastics transforms under UV light and how it contributes to the formation of harmful disinfection byproducts during water chlorination. They found that UV exposure changed the chemical composition of the microplastic-derived organic matter, affecting its reactivity during disinfection. The findings suggest that microplastics in water sources may indirectly increase the formation of potentially harmful chemicals during standard water treatment.
Leaching of organic matter from microplastics and its role in disinfection by-product formation
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Researchers found that microplastics leach organic matter into water that subsequently acts as a precursor for disinfection by-products during chlorination, with polystyrene MPs generating the most leachate and producing the most by-products compared to polyethylene MPs.
Mechanistic insight into the role of typical microplastics in chlorination disinfection: Precursors and adsorbents of both MP-DOM and DBPs
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Chlorination of polypropylene and polystyrene microplastics released dissolved organic matter that formed disinfection by-products, with PS-MPs being more susceptible to chlorination; the study found that even small MPs in drinking water can contribute to DBP precursor loads during treatment.
Comparison of chlorination resistance of biodegradable microplastics and conventional microplastics during the disinfection process in water treatments
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