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Poly(lactic acid) (PLA)/poly(butylene succinate adipate) (PBSA) films with Micro fibrillated cellulose (MFC) and cardanol for packaging applications

Cellulose 2024 16 citations ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count. Score: 50 ? 0–100 AI score estimating relevance to the microplastics field. Papers below 30 are filtered from public browse.
Annalisa Apicella, Giovanna Molinari, Vito Gigante, Arianna Pietrosanto, Loredana Incarnato, Laura Aliotta, Andrea Lazzeri

Summary

Researchers developed biodegradable packaging films by blending PLA and PBSA polymers with micro fibrillated cellulose, using cardanol as a bio-based dispersing agent. The resulting films showed improved mechanical and barrier properties compared to the base blend. The study presents a promising approach for creating sustainable food packaging alternatives that could help reduce reliance on conventional non-biodegradable plastics.

Polymers

Abstract Micro Fibrillated Cellulose (MFC) has emerged as a promising component in film formulations due to its unique barrier prope.rties. In this study, to best of our knowledge, cardanol, a biobased plasticizer derived from cashew processing, was employed for the first time, as a dispersing aid for MFC, during a liquid assisted extrusion technique with a Poly(lactic acid) (PLA)/Poly(butylene succinate adipate) (PBSA) blend. The aim of the work is the production of PLA/PBSA/MFC films for packaging applications. The addition of different MFC amount was investigated (added at 0.5, 0.75 and 1 wt.% concentrations). The results obtained are very interesting, in fact from one hand Cardanol improved the compatibility between PLA and PBSA and avoided the MFC agglomeration. On the other hand, micro fibrillated cellulose ensured a stable film blowing and the achievement of enhanced barrier properties, seal ability and mechanical resistance. In particular, the best result was obtained with an MFC content of 0.75 wt.% for which a good compromise in terms of films ductility, barrier properties and seal ability was achieved.

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