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Advances and Gaps in Real-Time Chemical Sensor Systems for Safeguarding U.S. Water Supplies from Emerging Contaminants
Summary
This review of 24 studies finds that new real-time sensors can quickly detect heavy metals and other contaminants in tap water, which could help catch pollution problems faster than current lab testing. But there's a major gap: sensors for PFAS ("forever chemicals," found in nonstick cookware and many everyday products) still aren't sensitive enough to detect these chemicals at the low levels the EPA considers safe. This matters because until better detection technology is developed and tested in real-world water systems, we may be missing harmful PFAS contamination in our drinking water.
Abstract : Emerging contaminants including per- and polyfluoroalkyl substances (PFAS), pharmaceuticals, microplastics, and heavy metals pose escalating threats to drinking water safety in the United States. Conventional laboratory-based monitoring methods lack the temporal resolution and rapid response capabilities needed for effective early warning and contamination prevention, creating critical vulnerabilities in water safety infrastructure. This systematic review synthesizes recent advances in real-time chemical sensor technologies for detecting emerging contaminants in drinking water systems. It involves evaluating their analytical performance, field deployment readiness, and translation potential for protecting public water supplies. Following PRISMA guidelines twenty-four (24) studies were analyzed encompassing electrochemical, optical, biosensor, microfluidic, and integrated IoT-based sensing platforms. Data extraction focused on sensor types, target analytes, analytical performance metrics, deployment contexts, and identified limitations. Electrochemical sensors demonstrated detection limits ranging from ng/L to µg/L for heavy metals and arsenic with response times under 10 minutes. Optical methods including surface-enhanced Raman spectroscopy achieved ultra-sensitive detection (pg/L to ng/L) but faced substrate reproducibility challenges. A critical gap emerged in PFAS detection, where current sensors fall 2-3 orders of magnitude short of EPA's 4 ng/L health advisory levels. Field deployment remained limited, with fewer than 30% of technologies reporting real-world testing. Biofouling, calibration drift, and matrix interference emerged as universal challenges. Real-time sensor technologies show considerable progress for heavy metal monitoring and integration with smart water systems. Critical gaps remain in ultra-trace contaminant detection, field validation, and regulatory acceptance pathways. Achieving PFAS detection at regulatory levels represents the most urgent research priority. Successful translation requires coordinated efforts in anti-fouling innovation, standardization, long-term field studies, and policy framework development.