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Upcycling of waste polyesters for the development of a circular economy
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This review surveys emerging chemical recycling and upcycling technologies for waste polyesters, particularly PET, covering thermal, photocatalytic, electrocatalytic, and biocatalytic depolymerization methods that convert plastic waste back into valuable monomers and chemicals to support a circular carbon economy.
The rapidly increasing production and widespread application of plastics have brought convenience to our lives, but they have consumed a huge amount of nonrenewable fossil energy, leading to additional CO2 emissions and generation of an enormous amount of plastic waste (also called white pollution). Chemical recycling and upcycling of waste plastic products (also called waste plastic refineries) into recycled monomers and/or valuable chemicals can decrease the dependence on fossil energy and/or reduce the emission of CO2, enabling the full utilization of carbon resources for the development of a circular economy. Polyesters, a vital class of plastics, are ideal feedstocks for chemical recycling due to the easily depolymerizable ester bonds compared to polyolefins. Among them, polyethylene terephthalate (PET) is the most widely used product, making its chemical recycling to a circular carbon resource a hot topic with significant concerns. In this feature article, recent progress in depolymerization of waste polyesters (PET and/or PET-containing materials) and the subsequent upgrading of depolymerized monomers (or intermediates) to valuable chemicals was reviewed and prospected. Newly reported technologies, such as thermal catalysis, photocatalysis, electrocatalysis, and biocatalysis, were discussed. The achievements, challenges, and potential of industrial applications of chemical recycling of polyesters were addressed.
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This review surveys advances in chemical recycling of polyethylene terephthalate (PET)—including glycolysis, hydrolysis, enzymatic depolymerization, and tandem catalysis—as strategies to recover monomers and close the plastic carbon loop. Since PET is a major source of microplastic pollution through bottle and textile degradation, effective chemical recycling pathways are critical for reducing its long-term environmental persistence.
Towards carbon neutrality: Sustainable recycling and upcycling strategies and mechanisms for polyethylene terephthalate via biotic/abiotic pathways
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This review maps both biological and chemical pathways for recycling and upcycling polyethylene terephthalate (PET), cataloging over 25 value-added products that can be derived from PET waste—including adipic acid, vanillin, and glycolic acid—and outlining how combining microbial depolymerization with advanced catalysis could support a lower-carbon circular economy.
Chemical Recycling and Upcycling of Plastic Waste: from Linear to Circular Economy
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Right now, only about 9% of plastic waste actually gets recycled, and most of what does get recycled turns into lower-quality material—not a real solution to the mountains of plastic piling up in our environment (and breaking down into the microplastics we're increasingly finding in our bodies). This review rounds up newer "chemical recycling" methods that can break plastic waste down to its molecular building blocks and even transform it into useful products like lubricants, offering a more promising path to actually reusing plastic instead of just downgrading it. These technologies are still working through real challenges like cost and efficiency before they can make a major dent in the plastic p
Chemical Recycling and Upcycling of Plastic Waste: from Linear to Circular Economy
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This review paper rounds up scientific progress on turning plastic waste into new chemicals and materials—instead of just melting it down into lower-quality plastic (what most "recycling" does today, and only for 9% of waste). Better recycling methods matter for your health because plastic that isn't properly processed often ends up in landfills, oceans, or breaking down into microplastics that contaminate our food, water, and even our bodies. These emerging chemical methods could help close the loop on plastic waste, though the researchers note real challenges remain before this happens at scale, including cost and technical hurdles.
Upcycling of PET waste: from one polymer to another polymer
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This study investigated microplastic distribution in coral reef sediments and reef-building coral tissues, documenting plastic particle accumulation in a biodiversity hotspot. The findings reveal that microplastics concentrate in reef systems and are ingested by corals, potentially interfering with filter feeding and causing tissue inflammation.
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