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Beyond Mechanical Recycling: Giving New Life to Plastic Waste

Angewandte Chemie International Edition 2020 1657 citations ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count. Score: 50 ? 0–100 AI score estimating relevance to the microplastics field. Papers below 30 are filtered from public browse.
Bert M. Weckhuysen, Ina Vollmer, Michael J. F. Jenks, Florian Meirer Florian Meirer Florian Meirer Mark Roelands, Florian Meirer Florian Meirer Bert M. Weckhuysen, Robin J. White, Ina Vollmer, Bert M. Weckhuysen, Toon van Harmelen, Bert M. Weckhuysen, Ina Vollmer, Ina Vollmer, P.J. de Wild, Bert M. Weckhuysen, Florian Meirer Bert M. Weckhuysen, Bert M. Weckhuysen, G. van der Laan, Ina Vollmer, Florian Meirer Florian Meirer Florian Meirer Florian Meirer Florian Meirer Ina Vollmer, Florian Meirer Jos T. F. Keurentjes, Florian Meirer Florian Meirer Jos T. F. Keurentjes, Bert M. Weckhuysen, Bert M. Weckhuysen, Florian Meirer Bert M. Weckhuysen, Florian Meirer

Summary

This review examines chemical recycling processes — including pyrolysis, solvolysis, and gasification — as alternatives to mechanical recycling for plastic waste, comparing their technical readiness, environmental performance via life-cycle analysis, and commercial development status.

Increasing the stream of recycled plastic necessitates an approach beyond the traditional recycling via melting and re-extrusion. Various chemical recycling processes have great potential to enhance recycling rates. In this Review, a summary of the various chemical recycling routes and assessment via life-cycle analysis is complemented by an extensive list of processes developed by companies active in chemical recycling. We show that each of the currently available processes is applicable for specific plastic waste streams. Thus, only a combination of different technologies can address the plastic waste problem. Research should focus on more realistic, more contaminated and mixed waste streams, while collection and sorting infrastructure will need to be improved, that is, by stricter regulation. This Review aims to inspire both science and innovation for the production of higher value and quality products from plastic recycling suitable for reuse or valorization to create the necessary economic and environmental push for a circular economy.

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