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Synthesis and analysis of lactose polyurethanes and their semi-interpenetrating polymer networks

International Journal of Polymer Analysis and Characterization 2022 2 citations ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count.
H. N. Cheng, Atanu Biswas, Sanghoon Kim, Michael Appell, Roselayne Ferro Furtado, Maria do Socorro Rocha Bastos, Carlúcio Roberto Alves

Summary

Researchers synthesized bio-based polyurethanes from lactose and toluene-2,4-diisocyanate using both conventional and microwave heating, then formed semi-interpenetrating polymer networks by combining these with poly(vinyl pyrrolidone) or poly(lactic acid). Microwave synthesis reduced reaction times and energy use, and the resulting materials were characterized as sustainable, agro-derived alternatives to fossil-based plastics.

In view of growing public awareness of environmental pollution, plastic waste, and microplastics, agro-based materials are increasingly used to replace raw materials derived from fossil feedstocks in order to take advantage of their sustainability, eco-friendliness, better recyclability, and lack of toxicity. One of our focal areas is lactose, which is the natural disaccharide found in milk; it is inexpensive and widely available. In this work, we synthesized polyurethanes from lactose and toluene-2,4-diisocyanate (TDI), using both conventional heat and microwave. Microwave was found to reduce the reaction time and save energy relative to conventional heat. Moreover, semi-interpenetrating polymer networks were made with a second polymer {e.g., poly(vinyl pyrrolidone) and poly(lactic acid)} in order to impart additional properties to the lactose-based polyurethanes. The resulting polymers were characterized with appropriate analyses.

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