0
Article ? AI-assigned paper type based on the abstract. Classification may not be perfect — flag errors using the feedback button. Tier 2 ? Original research — experimental, observational, or case-control study. Direct primary evidence. Sign in to save

Quick-Release Antifouling Hydrogels for Solar-Driven Water Purification

ACS Central Science 2023 33 citations ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count.
Xiaohui Xu, Néhémie Guillomaitre, Kofi S. S. Christie, R. Kōnane Bay, Navid Bizmark, Sujit S. Datta, Zhiyong Jason Ren, Rodney D. Priestley

Summary

Scientists created a loofah-inspired hydrogel material that uses sunlight to purify contaminated water at a rate of about 26 kilograms per square meter per hour, enough to meet daily drinking water needs. The material resists fouling and can produce clean water from various contaminated sources including those containing microplastics and heavy metals. This solar-powered approach offers a sustainable, off-grid solution for water purification in areas lacking conventional infrastructure.

Hydrogels are promising soft materials for energy and environmental applications, including sustainable and off-grid water purification and harvesting. A current impediment to technology translation is the low water production rate well below daily human demand. To overcome this challenge, we designed a rapid-response, antifouling, loofah-inspired solar absorber gel (LSAG) capable of producing potable water from various contaminated sources at a rate of ∼26 kg m-2 h-1, which is sufficient to meet daily water demand. The LSAG-produced at room temperature via aqueous processing using an ethylene glycol (EG)-water mixture-uniquely integrates the attributes of poly(N-isopropylacrylamide) (PNIPAm), polydopamine (PDA), and poly(sulfobetaine methacrylate) (PSBMA) to enable off-grid water purification with enhanced photothermal response and the capacity to prevent oil fouling and biofouling. The use of the EG-water mixture was critical to forming the loofah-like structure with enhanced water transport. Remarkably, under sunlight irradiations of 1 and 0.5 sun, the LSAG required only 10 and 20 min to release ∼70% of its stored liquid water, respectively. Equally important, we demonstrate the ability of LSAG to purify water from various harmful sources, including those containing small molecules, oils, metals, and microplastics.

Share this paper