Quantifying microplastic residence times in lakes using mesocosm experiments and 1D random walk model

Microplastic residence time in lakes is governed by complex and interrelated processes. In this work, we have used a series of in-lake mesocosm experiments combined with random walk modeling to understand microplastic residence times in the lake water column. Three size ranges of green fluorescent microplastic (1-5, 28-48, and 53-63 µm) were added to a 12m deep mesocosm and detected using fluorescence detectors. Experiments were conducted over one year capturing thermal stratification in summer as well as lake turnover in autumn. The measured residence times in summer ranged between ~1 and 24 days and depended mainly on particle size. The modeled residence time for the smallest particles (>200d) was considerably longer than the measured residence times in the mesocosm (~24d). This could be due to interactions between the small microplastic particles and existing particles in the lake. In contrast, during lake turnover large Rayleigh numbers showed that instabilities in the water column likely led to turbulent convective mixing and rapid sinking within the mesocosm.