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Modeling of heteroaggregation driven buoyant microplastic settling: Interaction with multiple clay particles
Summary
Researchers developed a mathematical model for the heteroaggregation of buoyant microplastics with multiple clay particles, addressing the limitation of existing single-clay-particle models that cannot accurately simulate settling behavior of low-density plastics. The model improves prediction of vertical microplastic migration in aquatic environments by accounting for interactions with multiple clay particles simultaneously.
The ecological risk of microplastics (MPs) has received widespread attention, but understanding ecological risk starts with understanding environmental migration. Heteroaggregation is an important process that affects the vertical migration of MPs, and the mathematical model is a common tool used to project the migration behavior of MPs. However, the mathematical model based on the aggregation of MPs with one clay particle is not applicable to simulate the migration behavior of buoyant microplastic (BMP). Hence, this study developed a model for heteroaggregation of one BMP with multiple clay particles based on the Population Balance Equation, and the main factors affecting the sedimentation of BMP are clarified through parameter sensitivity analysis and scenario simulation. The results show that neglecting the interaction of one BMP with multiple clay particles in the mathematical model can underestimate the predicted settling concentration of BMP, especially in aqueous environments with higher clay concentration and salinity. The settling process of BMP is controlled by the heteroaggregation rate, which is sensitive to environmental conditions and insensitive to particle properties. This study emphasizes the importance of considering the interaction of one BMP with multiple clay particles in the future mathematical model, which will provide a more reliable prediction of the migration of MPs in aquatic environments.