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Influence of Green Nanofillers on the Morphological, Mechanical Properties, and Degradation Kinetics of <scp>PBS</scp>/<scp>PBAT</scp> Blends: A Potential Sustainable Strategy for Fisheries Applications

Journal of Applied Polymer Science 2025 1 citation ? Citation count from OpenAlex, updated daily. May differ slightly from the publisher's own count. Score: 43 ? 0–100 AI score estimating relevance to the microplastics field. Papers below 30 are filtered from public browse.
Yousra Nait Hamou, Mostapha Benomar, Yousra Nait Hamou, Mostapha Benomar, Yousra Nait Hamou, Yousra Nait Hamou, Samira Benali, Mostapha Benomar, Mostapha Benomar, Samira Benali, Samira Benali, Mostapha Benomar, Samira Benali, Mostapha Benomar, Samira Benali, Mostapha Benomar, Jean‐Marie Raquez Samira Benali, Mostapha Benomar, Samira Benali, Jean‐Marie Raquez Samira Benali, Sandro Gennen, Jean‐Michel Thomassin, Samira Benali, Samira Benali, Samira Benali, Jean‐Marie Raquez Jean‐Marie Raquez Jean‐Marie Raquez Jean‐Marie Raquez Jean‐Michel Thomassin, Job Tchoumtchoua, Job Tchoumtchoua, Samira Benali, Jean‐Marie Raquez Job Tchoumtchoua, Jean‐Marie Raquez Job Tchoumtchoua, Jean‐Marie Raquez Hassan Er‐Raioui, Hassan Er‐Raioui, Hassan Er‐Raioui, Hassan Er‐Raioui, Mostapha Benomar, Jean‐Marie Raquez Jean‐Marie Raquez Jean‐Marie Raquez Jean‐Marie Raquez Mostapha Benomar, Jean‐Marie Raquez Jean‐Marie Raquez

Summary

Researchers developed biodegradable polymer blends reinforced with nanochitin and nanocellulose — materials derived from natural sources — as a potential replacement for synthetic nylon fishing nets. The bio-based nanofillers improved the mechanical strength and altered degradation rates of the PBS/PBAT blends, bringing performance closer to what is needed for real fishing applications. Replacing synthetic nylon with biodegradable alternatives could meaningfully reduce ghost fishing and the microplastic pollution that comes from fragmenting nets in the ocean.

Polymers

ABSTRACT Synthetic nylon fishing nets pose significant threats to marine ecosystems, contributing to ghost fishing and microplastic pollution. While the development of biodegradable polymers for marine applications has progressed, significant challenges remain in achieving the mechanical performance required for fishing nets, particularly under water conditions. This study addresses these challenges by investigating the incorporation of nanochitin and nanocellulose fillers into PBS/PBAT blends, aiming to optimize their mechanical properties and to control the degradation behavior for marine environments. First, various PBS/PBAT nanocomposites were prepared with chitin and cellulose nanofillers, and tensile tests identified the most effective fillers for mechanical reinforcement. Differential scanning calorimetry (DSC), size exclusion chromatography (SEC), and scanning electron microscopy (SEM). The results demonstrated significant mechanical reinforcement in air conditions, with efficient nanofiller dispersion, particularly in two nanocomposites: PBS/PBAT/ChNCsLac 1% and PBS/PBAT/NFCEster 1% . These formulations exhibited notable improvements in mechanical properties compared to the other blends. Specifically, Young's modulus increased by +15% and + 22%, respectively, while elongation at break improved by +10% and + 7%, respectively. Under aqueous conditions, PBS/PBAT/ChNCsLac 1% also showed a remarkable +52% increase in elongation at break. Additionally, weathering tests were also examined the nanofillers' influence on degradation kinetics, revealing that chitin nanofillers accelerated degradation under controlled conditions. These findings suggest that while nanochitins and nanocelluloses improve mechanical properties in certain environments, further research is required to optimize their performance in water.

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