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Sedimentation and shear-induced dynamics of spheroids in fluids with spatial viscosity variations
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Researchers used a generalized reciprocal theorem approach to analytically model how spheroid-shaped particles—relevant to elongated microplastics—settle and rotate in viscosity-stratified fluids. The analysis provides theoretical predictions for how viscosity gradients in natural water columns affect the transport dynamics of non-spherical microplastic particles.
A generalized reciprocal theorem is used to relate the force and torque induced on a particle in an inertia-less fluid with small variation in viscosity to integrals involving Stokes flow fields and the spatial dependence of viscosity. These resistivity expressions are analytically evaluated using spheroidal harmonics and then used to obtain the mobility of the spheroid during sedimentation, and in linear flows, of a fluid with linear viscosity stratification. The coupling between the rotational and translational motion induced by stratification rotates the spheroid’s centerline, creating a variety of rotational and translational dynamics dependent upon the particle’s aspect ratio, $\kappa$ , and the component of the stratification unit vector in the gravity direction, $d_g$ . Spheroids with $0.55\lessapprox \kappa \lessapprox 2.0$ exhibit the largest variety of settling behaviors. Interestingly, this range covers most microplastics and typical microorganisms. One of the modes include a stable orientation dependent only on $\kappa$ and $d_g$ , but independent of initial orientation, thus allowing for the potential control of settling angles and sedimentation rates. In a simple shear flow, cross-streamline migration occurs due to the stratification-induced force generated on the particle. Similarly, a particle no longer stays at the stagnation point of a uniaxial extensional flow. While fully analytical results are obtained for spheroids, numerical simulations provide a source of validation. These simulations also provide additional insights into the stratification-induced force- and torque-producing mechanisms through the stratification-induced stress, which is not accessed in the reciprocal theorem-based analytical calculations.
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